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<!--StartFragment--><p class="MsoTitle" style="text-align: center;margin-right: -0.5in; "><b><span style="font-family:"Times New Roman""><font size="4">Seminar on</font></span></b></p><p class="MsoNormal" align="center" style="text-align:center"><font size="4"><b><span style="letter-spacing: 1.5pt; ">Modern Optics and Spectroscopy</span></b><span style="font-family:Arial;
letter-spacing:1.5pt"><o:p></o:p></span></font></p><p class="MsoNormal"><b><span style="font-family: Arial; letter-spacing: 1pt; "><font size="4"> </font></span></b></p><p class="MsoNormal" align="center" style="text-align:center"><b><i><span style="letter-spacing: 1pt; "><font size="4">Creating beakers without
walls: <o:p></o:p></font></span></i></b></p><p class="MsoNormal" align="center" style="text-align:center"><b><i><span style="letter-spacing: 1pt; "><font size="4">Formation of deeply-supercooled
binary liquid solutions from nanoscale amorphous solid films</font></span></i></b></p><div><br></div><p class="MsoNormal" align="center" style="text-align:center"><b><span style="letter-spacing: 1pt; "><font size="4">Bruce D. Kay,<o:p></o:p></font></span></b></p><p class="MsoNormal" align="center" style="text-align:center"><span style="letter-spacing: 1pt; "><font size="4">Pacific
Northwest National Laboratory</font></span><span style="font-size: large; letter-spacing: 1pt; "> </span></p><p class="MsoNormal" align="center" style="text-align:center"><span style="letter-spacing: 1px; "><font size="4">Tuesday, Decemeber 3, 2013</font></span></p><p class="MsoNormal" align="center" style="text-align:center"><span style="font-family: Times; "><font size="4">12:00-1:00p.m. </font></span></p><p class="MsoNormal"><br></p><p class="MsoNormal" style="text-align:justify"><font size="4">Supercooled
liquids are metastable and their lifetimes are dictated by the kinetics for
crystallization. Traditional experimental studies have used a variety of
methods to suppress crystallization while cooling from the liquid phase. An alternate
approach is to heat an amorphous solid above its glass transition temperature,
Tg, whereupon it transforms into a deeply-supercooled liquid prior to
crystallization. We employ molecular beams, programmed desorption (both TPD and
isothermal), FTIR vibrational spectroscopy, and rare gas permeation to
synthesize and characterize compositionally tailored nanoscale films of glassy
methanol and ethanol. We demonstrate that these films exhibit complete
diffusive intermixing and suppressed crystallization when heated above
Tg. Furthermore, the resulting container-less liquids evaporate as
continuously mixed ideal binary solutions while retaining their solid-like
macroscopic shapes. This approach provides a new method for preparing
deeply-supercooled liquid solutions in metastable regions of their phase
diagram and for studying the kinetics of their phase separation and
crystallization as they approach thermodynamic equilibrium. The applicability
of this technique for studying aqueous liquid solutions will also be presented
and discussed.<o:p></o:p></font></p><p class="MsoNormal"><font size="4"> </font></p><p class="MsoNormal" align="center" style="text-align:center"><font size="4">Grier Room, MIT Bldg 34-401<o:p></o:p></font></p><p class="MsoNormal" align="center" style="text-align:center"><font size="4">Refreshments served after
the lecture</font><font size="6"><o:p></o:p></font></p>
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